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Frustrated antiferromagnets

 

Theoretical studies of quantum models of low-dimensional magnetic solids reveal surprising new features and explain properties of newly synthesized materials.
REAL MAGNETIC MATERIALS exhibit a macroscopic quantum state in which the atomic moments interact through quantum-mechanical 'exchange forces'. These result from overlap of atomic wave functions and can favour parallel (ferromagnetic) or antiparallel (antiferromagnetic) alignment of moments. The low energy states then minimise the sum of all pair interactions, and, because of geometrical constraints, not all pairs can adopt their lowest energy state. This is termed frustration, and can lead to complex magnetic structures as well as complete breakdown of magnetic order.

During 1999 we have continued a program of study of such systems, based on both analytic and numerical techniques. Some of the completed work includes:

  • a study of the low energy excited states of the J1-J2 model (square lattice with first and second interactions) in the quantum disordered "spin-liquid" phase

  • strong evidence that the ground state in the same region has dimer order with striped correlations. This may be related to the striped phases observed experimentally in the cuprate superconductors

  • the first detailed theoretical study of the magnetic structure and phase diagram of the quasi-two-dimensional material SrCu2(BO3)2, found by a Japanese group in 1999.

 

Valeri Kotov, Jaan Oitmaa,
Oleg Sushkov & Wei Hong Zheng

 

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